Disclaimer: The question here has been solved, now:
(For jeapardy it is stated below, anyway. Have fun! ;) )
Summary: This is a summary of the discussions:
- Measures: Atom Definitions
- Borel Measures: Discrete & Continuous Definition?
- Borel Measures: Atoms vs. Point Masses
Reference: Further results are accessible from:
Definitions
Call a measure discrete if it is discretely concentrated: $$\mu(\Omega\setminus\Delta)=0\quad(\#\Delta\leq\aleph_0)$$ and continuous if any discrete has no mass: $$\#\Delta\leq\aleph_0\implies\mu(\Delta)=0$$ (Note that I do not require it to decompose into singletons for reason.)
Call a measure atomic if is made out of atoms only: $$\mu(\Omega\setminus\bigcup_{A\in\mathcal{A}} A)=0\quad(\mathcal{A}:\text{ atoms})$$ and atomless if it has no atoms at all: $$\mathcal{A}\text{ empty}\quad(\mathcal{A}:\text{ atoms})$$ (I have chosen these slightly different formulations for more clarity.)
Discussion
Now, consider a sigma-finite Borel measure $\lambda:\mathcal{B}(\Omega)\to\mathbb{R}_+$.
First, let it be discrete.
Then, by Zorn's lemma it splits into a finest measurable partition.
(See Proof to Finest Measurable Partition.)
These are all atoms and therefore it is atomic.
Conversely, let it be atomic.
Then, by sigma-finiteness atoms cannot have infinite mass.
(See Last Part of Proof to Measure Atoms: Definitions.)
Also, there are at most countably many disjoint ones.
However, they do not need to be countable themselve.
(See Example on Atoms vs. Point Masses.)
Luckily, for separable metric spaces every atom even shrinks to a point mass.
(See Proof by Nate Eldredge.)
Thus, it is concentrated on countable set and therefore discrete.
This completes the equivalence!
Remarks
Besides, note that the only measure that is both discrete and continuous is the trivial measure.
Similarly, the only measure that is both atomic and atomless is the trivial measure.
Problem
Is the first claim of the discussion really true?
Namely, every countable measure space admits a finest measurable partition: $$\#\Omega\leq\aleph_0:\quad\Omega=\bigsqcup_{k=1}^\infty A_k\quad(A_k\in\Sigma)$$