I'll brute force this. There are probably smarter ways though. Let's find the antiderivative.
$$\int\frac{t^2}{t^4}\text{ d}t-\int \frac{\sin^2(t)}{t^4} \text{ d}t$$
$$\implies -\frac1t-\frac12\int (1-\cos(2t))\cdot\frac1{t^4} \text{ d}t$$
$$\implies -\frac1t+\frac1{6t^3}-\frac12\underbrace{\int\frac{\cos(2t)}{t^4} \text{ d}t}_A$$
Okay, let's solve $A$. We can integrate by parts, with $u$(derivative side) being the trig function and $v$(integral side) being the denominator. You can quickly calculate this using tabular, and we get $$A=-\frac1{3t^3}\cos(2t)+\frac{1}{3t^2}\sin(2t)+\frac2{3t}\cos(2t)+\frac43\operatorname{Si}(2t)$$
where Si is the sine integral.
Hence the full antiderivative is $$I(t)=-\frac1t+\frac1{6t^3} -\frac1{6t^3}\cos(2t)+\frac{1}{6t^2}\sin(2t)+\frac1{3t}\cos(2t)+\frac23\operatorname{Si}(2t)$$
We now need to take two limits, first to $0$, then to $\infty$.
$$\lim_{t\to0}I(t)=0$$ It's very very bashy so I'll use words to describe it in case you want to work this out (probably not).
We find this by splitting the Si out first, that goes to $0$. Write every other term in a common denominator, use le hospital rule. Now, you would take out several terms using addition rule, spam le hospital and you have the answer.
$$\lim_{t\to\infty}I(t)=\frac{\pi}3$$ For this one, completely split every term via addition rule. The only term that gives a value is the Si term, which spits out our limit value.
We now have shown your integral is $$\int^{\infty}_0\frac{t^2-\sin^2(t)}{t^4} \text{ d}t=\frac{\pi}3$$
this is a dumb method ig, there's probably much smarter ones like the lapalce one noted in the comments or some other stuff