[Update. Having thought about this even more I think it makes sense to expand on my original remarks.]
I've been thinking about this question for a bit, and I've realized a few things.
Basis-free vs chart-free
First, we have clarify what we mean by "coordinate free". A choice of coordinates entails a choice of a local chart, i.e., parametrization by a vector space, and a choice of a (ordered) basis for that vector space.
So we can ask for basis-free approaches, or more ambitiously, chart-free approaches.
Implicit vs explicit
We have to temper our expectations a little bit, as the definition of a manifold defines it in terms of charts. Moreover, even if we have no privileged basis, the definition of an $n$-dimensional vector space is that it has a basis of cardinality $n$. Thus we are going to be implicitly using facts about charts and bases no matter what we do.
(A clever topologist might propose circumventing the second point by defining charts to be parametrized by arbitrary topological vector spaces of topological dimension $n$, but they would struggle mightily to establish much useful about these spaces without accidentally proving the existence of a basis along the way.)
However, what we can ask for are approaches which avoid explicitly invoking charts and/or bases.
There are two approaches that I think work well to this end - a more concrete one that is basis-free but invokes charts, and a more abstract one that eschews either.
Concrete basis-free approach using charts
We will avoid explicit invocation of a basis for the integral, but as per previous remarks, we must use some fact about finite dimensionality somewhere under the hood, and we do so by establishing, via well known linear algebra facts, that the signed volume of an $n$-vector is independent of its representation.
Let $V$ be an $n$-dimensional oriented vector space, $\mu$ a
translation invariant measure on $V$, and let $v_1\wedge\cdots\wedge v_n =
w_1\wedge\cdots\wedge w_n \in \Lambda^n(V)$, the $n$-th exterior product. Then
the signed $\mu$-volumes of the parallelepipeds $(v_1,\cdots,v_n)$ and
$(w_1,\cdots,w_n)$ are equal.
This immediately leads to the following definition:
Let $V$, $\mu$ be as above. The signed $\mu$-volume $\operatorname{vol}_\mu(\lambda)$ of an $n$-vector $\lambda\in\Lambda^n(V)$ is given by the signed $\mu$-volume of any (hence every) parallelepiped $(v_1,\cdots,v_n)$ such that $\lambda=v_1\wedge\cdots\wedge v_n$.
Having adopted this notion of signed volume, we may develop the theory of integration without ever touching $\mathbb R^n$, nor any basis, again. For now the integral is uniquely determined by linearity on differential forms and the following two requirements.
- For every orientation preserving diffeomorphism $f\colon M\to N$ and $\omega\in \Omega^n(N)$ we have:
$$\int_M f^*\omega = \int_{N}\omega\text{.}$$
- For every $n$-dimensional oriented vector space $V$, $U\subseteq V$ open, translation invariant measure $\mu$ on $V$, nonzero $n$-vector $\lambda\in\Lambda^n(V)$, and $\omega\in \Omega^n(U)$ we have:
$$\int_U \omega = \frac{\int_{U} \langle \omega(p),\lambda \rangle d\mu(p)}{\operatorname{vol}_\mu(\lambda)}\text{.}$$
We do still need to invoke partitions of unity at some point in our development of the theory of forms, but these partitions of unity can be supported on charts parametrized by arbitrary vector spaces, with no privileged bases.
Abstract chart-free approach via Stokes
The preceding approach was still concrete in that it told us, albeit in a basis-free manner, directly how to compute the integral over a chart, from which a partition of unity then shows us how to compute it explicitly in the general case.
We now consider a more abstract approach, via Stoke's theorem, and the natural $\sigma$-algebra of measurable sets that our manifold is equipped with. Although no measure is defined, it is still equipped with a natural sub-algebra of null-sets. Under the hood, these algebras come from local charts, but from them we get a number of interesting properties that can then be discussed without appealing to charts directly.
Of particular use is the fact that, for any locally finite measure $\mu$ on $M$, if $A\subset M$ is measurable, then $\mu(A)$ approximated by $\mu(\overline{U})$, where $U$ is open with smooth boundary.
This is inherited from the charts, where it follows from a Vitali covering theorem, for example.
That fact implies that if an integration operator is to linearly and continuously map compactly supported $n$-forms to measures, then it is completely determined by integration over open sets with smooth boundary.
Moreover, from partitions of unity and the local theory of forms, a compactly supported $n$-form can be decomposed into terms of the form $\phi d\nu$, where $\nu$ is an $(n-1)$-form.
The upshot is that an integration operator is completely determined by its action on forms $\phi d\nu$, and with the help of step functions approximating $\phi$, that action is determined via integrals of the form $$\int_U d\nu\text{,}$$ where $U\subseteq M$ is an open subset of smooth boundary.
But this means we can "define" integration inductively, saying in dimension $0$ that integration of a function over a singleton is given by the evaluation map, and in higher dimensions we define
$$\int_U d\nu:=\int_{\partial U}\nu\text{,}$$
for every open $U\subseteq M$ with smooth boundary.
Per our remarks, this uniquely determines the integral operator. Now, the question of existence of such an operator is a thornier issue, as the above "definition" might not be a priori well-defined.
Still, this gives a chart-free characterization of the integral as the only integration operator, if one exists, that both satisfies Stokes, and acts as evaluation in dimension $0$.
One could use this "Stokes" approach to characterize the integral, and then establish existence through the previously mentioned basis-free approach using charts.