Supposing if a problem with $n$ non-deterministic bits is in $O(2^{\alpha n})$ time at every $\alpha\in(0,1)$ then is there evidence that problem can or cannot be $\mathsf{NP}$-complete?
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Yes, such problems can be NP-complete.
Consider classical NP-complete graph problems like clique.
Clique has an $O(2^n)$ time algorithm, where $n$ is the number of vertices. However the input for clique is the adjacency matrix of the graph, which has $n^2$ bits. Therefore when the size of input is measured in bits, clique has an $O(2^\sqrt{n})$ time algorithm, which is $O(2^{\alpha n})$ for any positive $\alpha$.
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