One of the best ways to get a handle on a group is to recognize it as isomorphic to a set of symmetries of some structure. The dihedral group of order $2n$ is easily recognized as the set of symmetries of a regular $n$-gon, the symmetric group as the permutations of a set, the Klein-four group as the symmetries of the 'cross'---one pair of opposing prongs are longer than the other pair.
The previous descriptions are also in a sense 'exhaustive': every 'sensible' symmetry you could conceive of those structures is represented by some element of the group. An example where the group is not exhaustive over its structure is $C_n$ over the regular $n$-gon (reflection is missing), or $A_n$ over the set of $n$ elements.
I wish to know of a structure that a free group---specifically $F_2$---naturally acts on which it is also in a sense 'exhaustive'. I'm aware of $F_2$'s Cayley graph, but I want other examples.
EDIT
The question may have been a bit unfair and imprecise, but I can't help that it is really. One of the reasons it may be unfair is that 'exhaustive' is a bit subjective. For example, I myself cannot point out a structure that $C_n$ naturally acts on that $D_{2n}$ could not be conceived of as acting on also; however, both of these groups also sit in $S_n$ in a more-or-less canonical fashion. But there are structures, such as polygons, that we think of as $D_{2n}$ acting on naturally rather than $S_n$.
I'm trying to find structures such that when we think of their 'natural' set of symmetries, the group of these symmetries would be isomorphic to a free group. I want a couple of examples, as I'm slightly disappointed in having only the Cayley graph or finite tuples of words as a reference. Other groups have many examples of acting on a structure. For example the Klein four group could also be realized as the symmetries of a proper rectangle, $A_4$ can be realized as the rigid motions of the tetrahedron rather than the even permutations of a 4-element set.
I also don't want these examples to be 'cheap'. What I mean by this is that the action is not arrived at by quotienting by a normal subgroup to get an action that is more properly realized by another group.

